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Correspondence, manuscripts, memoranda, receipts, certificates, financial and legal documents, envelopes, clippings, pamphlets, and other printed materials dealing with social and family relationships, the sons' education, professions, and military careers, the Mexican-American War and the Civil War, real estate and financial matters, and with the deaths and bequests of various family members. Among the cataloged correspondents are: Alexander Hamilton, John Church Hamilton, Gen. Schuyler Hamilton, Ralph Isaacs Ingersoll, Charles Augustus Peabody, Gen. J. Fred Pierson, Gen. Winfield Scott, Martin Van Buren, and a manuscript by George Washington.

Correspondence, photographs, leaflets, pamphlets, manuals, reports and newsletters. Much of the correspondence details Marcu's efforts to persuade the American Military Government for Bavaria not to issue a weapons permit to a former Nazi who was seeking a position with the newly reconstituted police force.

Correspondence, manuscripts, documents, and newspapers. These include over four hundred letters to Alexander, as well as miscellaneous letters and telegrams; some of his manuscripts and notes; business records of his law firm; military documents of the western divisions of the Confederate Army; copybooks and letter books; and complete and partial newspapers and clippings from the various Southern newspapers (in particular THE SAVANNAH REPUBLICAN, the DAILY DISPATCH of Richmond, and the ADVERTISER AND REGISTER of Mobile) which carried Alexander's dispatches.

Letters written to Gay from political and literary contemporaries such as Horace Greeley, Charles Sumner, and William Bryant; reports in letter form from his reporters at the front during the Civil War; and personal correspondence including many letters from his wife, Elizabeth Neall Gay. Letters written to Mrs. Gay from family friends and business associates including many from her husband. Correspondence of other members of the Gay family including Walter Gay, Sarah Gay, and Allan Gay. Diaries, notebooks, and journals of Sydney Howard Gay.