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Henry Boynton Smith (1815-1877) was a Congregational Presbyterian minister, theologian, and Union Theological Seminary professor and librarian. The collection contains correspondence, clippings and scrapbooks, notebooks from his studies in Germany, notes for his courses as well as student notes, and sermons.

Philip Schaff (1819-1893) was a theologian, church historian, ecumenist, and Union Theological Seminary professor. Schaff was president of the American Bible Revision Committee, which he organized in 1871 at the request of the British Committee on Bible Revision. The collection contains correspondence, including from the American Bible Revision Committee and the British Committee on Bible Revision; notes and lectures; diaries; and scrapbooks and memorabilia, including a photograph album.

Thomas Samuel Hastings was a Presbyterian pastor of New York City and professor and president of Union Theological Seminary. The collection consists of correspondence, writings, and scrapbooks relating to activities of the seminary and the debate concerning the Presbyterian Creed. Included in the collection are also a notebook of his father, Thomas Hastings (1784-1872), and a travel diary that may be of his son, Thomas Hastings (1860-1920).

William Adams was a Presbyterian minister, pastoral theologian, UTS professor and president, and maternal grandfather of William Adams Brown. The collection contains bound "In Memoriam" books, as well as sermons written by Adams from the 1830s through the mid-1870s.