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This collection contains predominantly early 19th-century prints of architecture, cityscapes, and landscapes, with some ethnographic views, in the United Kingdom, continental Europe, and other selected countries. The majority of images are from published sources and are uncolored. Nearly all the prints are titled and most include artist, printer, and/or publisher information. Many noted printmakers are represented in this collection, most of whom were British.

Correspondence, manuscripts of poems, and manuscripts of lectures by Benjamin. The correspondence consists of original letters of Benjamin, typescript and photostatic copies of Benjamin letters in other libraries, and letters to Benjamin from some of his literary contemporaries including Paul Hamilton Hayne, Willis Gaylord Clark, John Lothrop Motley, and Fitz-Greene Halleck. Many of the letters relate to Park Benjamin's lecture tours. There are other family letters and many documents relating to the Benjamin family,and two letterbooks of John Lothrop Motley. Also, a large amount of genealogical material of the Benjamin family, and its related families from the 16th century to the present day. There are also financial records, monographs, clippings, and photographs.