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Correspondence, manuscripts, dispatches, documents, clippings and other printed materials concerning his career as an editor and correspondent for the New York Herald Tribune in Moscow, Berlin and New York, as a staff member of the Institute of Pacific Relations from 1932 to 1934, as deputy director in the Office of War Information overseas branch, 1941-44, as an owner and editor of the New York Star, 1948-49, as an instructor in communications at Sarah Lawrence College, 1950-1951, as a book editor at Simon and Schuster, Publishers, 1951-1970, and as an author and translator.

Correspondence, notes, articles, reports, and speeches of Gildersleeve, including materials relating to the United Nations Conference in San Francisco, 1945, the Dumbarton Oaks Conference, the International Federation of University Women, the American Association of University Women, the American Council on Education, and the Near East College Association. The most note-worthy item in the collection is a letter from President Franklin D. Roosevelt, appointing Dean Gildersleeve to serve as a member of the U.S. Delegation to the Charter Conference of the United Nations. The collection also contains some material relating to Barnard College affairs.