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The Chen Lifu papers (陳立夫檔案) mainly document his involvement in Chinese politics during the Republican era, dating from 1926 to 1989, with the bulk dates from 1926 to 1951. The papers consist of correspondence, portrait, meeting documents, reports, plans, speeches, writings, memoir, and printed materials. The papers focus on Chen Lifu's political career as the Head of the Central Bureau of Investigation and Statistics and the Minister of Education, as well as his general involvement in politics dating from 1926 to 1949.

The H. H. Kung papers document Dr. Kung's political career from 1936 to 1944. The bulk of the papers consist of correspondence and political documents during the time when he was serving as the Minister of Finance, the Governor of the Central Bank of China, and the Vice Premier of the Executive Yuan. Materials in the collection include correspondence, writings, speeches, documents, reports, and telegrams relating to the Xi'an Incident, Sino-Japanese War, financial situation in China during the war year, his involvement in foreign diplomacy, Executive Yuan, the KMT Central committee, etc.

The K.P. Chen papers documented the banking and finance career of a banker, entrepreneur, and finance advisor, Kwang Pu Chen dating from 1936 to 1968. Materials in the papers include accounts, loan contracts, correspondence, telegrams, diaries, financial reports, , letters, news clippings, notes, photographs, press releases, printed materials, and reports.

The Shih-hui Hsiung (Shihui Xiong) papers consist of materials documenting Hsiung's life and political career from 1907 to 1974. The highlights of the papers are the manuscripts, which include six volumes of Hsiung's memoir, seven volumes of diaries over 43 years, and approximately 440 original handwritten speech scripts. The photographs and political and military affairs related documents focus on Hsiung's active involvement in the northeast region and abroad from 1930 to 1948. The papers overall consist of correspondence, calligraphy scrolls, diaries, a diploma, documents, letter books, manuscripts of published and unpublished works, maps, newspaper clippings, notes, oversize military notices, poems, photographs, photograph albums, reports, and other materials.

The V. K. Wellington Koo papers document the diplomatic legacy of Wellington Koo as a Chinese statesman and diplomat of the 20th Century. The papers primarily consist of materials collected during Koo's diplomatic career, relating to the Lytton Commission, 1932-1933; the League of Nations, 1931-1940; the United Nations, 1944-1946; his ambassadorships to France, 1932-1941; to Britain, 1941-1946; to the United States, 1946-1956; as the Senior Advisor to the Republic of China from 1956; and as the Judge on the International Court of Justice, 1957-1966. The materials include correspondence, diaries, memoranda, manuscripts, documents, notes, speeches, maps, photographs, printed material, and audio visual material. The bulk of the materials emphasizes China's domestic and foreign affairs, such as the Sino-Japanese conflict, World War II and the Cold War in the Far East region, as well as the League of Nations and the United Nations.

The Zhang Fakui papers emphasize General Zhang's military career as a Chinese Nationalist General during the important years of the Sino-Japanese War. The bulk of the papers consist of documents and maps relating to the history of the Fourth War Zone which he commanded during the Sino-Japanese War dating from 1940 to 1947. Also included are documents related to the governance and development of the Hainan dating from 1939 to 1949. Materials include correspondence, documents, maps, photographs, reports, manuscripts, and diaries.