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Correspondence, manuscripts, dispatches, documents, clippings and other printed materials concerning his career as an editor and correspondent for the New York Herald Tribune in Moscow, Berlin and New York, as a staff member of the Institute of Pacific Relations from 1932 to 1934, as deputy director in the Office of War Information overseas branch, 1941-44, as an owner and editor of the New York Star, 1948-49, as an instructor in communications at Sarah Lawrence College, 1950-1951, as a book editor at Simon and Schuster, Publishers, 1951-1970, and as an author and translator.

Correspondence, memoranda, photographs, manuscripts, lists, legal and financial documents, and printed materials of Simon. The personal and business papers include correspondence with authors, inscribed photographs of authors, editorial files, files for his special art, photography, and music projects, correspondence files relating to Simon and Schuster, Inc., personal and family correspondence, documents, and photographs. Correspondents include Irving Berlin, Margaret Bourke-White, Henri Cartier-Bresson, Joseph E. Davies, Dwight D. Eisenhower, Philippe Halsman, Jerome Kern, Cole Porter, Kenneth Roberts, Arthur Schnitzler, Jerome Weidman, and Sloan Wilson.