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The collection contains correspondence with the authors, including contracts signed with authors as well as negotiations with the authors over various aspects of publishing their works; financial records documenting many aspects of the operation of Harper & Brothers, including royalties paid to authors, records of stock offerings and company reorganizations, and general ledgers which contain daily notes on all aspects of the operation of the business; book catalogues and trade lists; research materials collected by Eugene Exman for his history of Harper & Brothers; visual materials, from drawings and photographs of Harper's authors to colophon designs and an oil painting of the original Harper's building.

Thirty affectionate letters of Henry James to his close friend Ranee Margaret of Sarawak. Also, letters to Walter Berry, Howard V. Knox, and Theodora Sedgwick.

Letters addressed to the Cranes from various members of the Crane and Howorth families, and from prominent literary figures such as Joseph Conrad, Henry James, H.G. Wells, George Bernard Shaw, Hamlin Garland, Elbert Hubbard, and Rider Haggard. A number of these letters relate to Cora Crane's activities after Stephen Crane's death, but the majority have to do with life at Brede Place in Sussex. Also present are a number of holograph manuscripts of Stephen Crane's literary works and manuscripts and typescripts of other material which he dictated. There is a group of stories and articles by Cora Crane, some pictures, photographs, art, and memorabilia. Also, seventy-four books from Crane's library, many of them signed.