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The papers consist of correspondence, manuscripts, documents, original art works, bibliographic notes and material on exhibitions. There are letters from Aleksandr Benois, Mikhail Chekhov, Fedor Komissarzhevskiĭ, Georgiĭ Lukomskiĭ, Nikolaĭ Medtner, Vladimir Nabokov and Aleksandra Tolstai︠a︡, and one letter each from Ivan Bunin, Mikhail Fokin, Tyrone Guthrie, Sok Hurok and Serge Kusevit︠s︡kiĭ. The manuscripts include essays by Dobuzhinskiĭ on such topics as the Mir Iskusstva group, Pushkin's illustrations, Aleksandr Blok, Kuzḿa Petrov-Vodkin and Josʹe-Maria Sert. There are original art works (pen and ink, goache, etc.) relating to his artistic and theatrical productions. Also included are photographs of Russian scenes, apparently from before World War I.

This collection contains materials related to Chermayeff's personal, professional, and academic lives, the bulk originating during his residency in the United States, beginning in the late 1930s. Project records document the full range of his work, including many records from his British period. The collection also contains extensive correspondence with personal friends, clients, and professional and academic colleagues.