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Papers of the Jay family and of those families related to the Jay family, including Bruen, Butterworth, Chapman, Clarkson, Dawson, Du Bois, Field, Iselin, McVickar, Mortimer, O'Kill, Pellew, Pierrepont, Prime, Robinson, Schieffelin, Von Schweinitz, Sedgwick, and Wurts. In addition to family and personal matters, the correspondence deals with anti-slavery, New York State civil service, repeal of the Missouri Compromise, the Civil War, the Blair Bill, international affairs, and New York City and State politics and government. There are letters from numerous prominent persons including George Bancroft, F.A.P. Barnard, Bismarck, William Cullen Bryant, Aaron Burr, James Fenimore Cooper, Ralph Waldo Emerson, Hamilton Fish, Albert Gallatin, Horace Greeley, Nathaniel Hawthorne, Oliver Wendell Holmes, Washington Irving, Frances Anne Kemble, Jenny Lind, Henry W. Longfellow, Seth Low, James Russell Lowell, John Stuart Mill, Alice Duer Miller, Clement Clarke Moore, J.P. Morgan, Thomas Nast, Commodore Matthew Perry, Franklin D. Roosevelt, Theodore Roosevelt, Elihu Root, Carl Schurz, William H. Seward, William T. Sherman, Charles Sumner, and John Greenleaf Whittier.

Correspondence, documents and manuscripts from late seventeenth and eighteenth century France, especially from the French Revolution, collected by Sam Schaefler. Authors include J.B. Colbert Torcy and the Duchesse Du Lude. Many of the items from the French Revolution represent the work of the Committee of Public Safety and the Committee of General Security. French Revolutionary leaders represented in the collection include François-Antoine Boissy D'Anglas, Jean-Baptiste-Noel Bouchotte, Pierre Joseph Cambon, Lazare Carnot, Jean-Marie Collot D'Herbois, l'Abbʹe de Fauchet, Philippe-Antoine Merlin de Douai, Jean Victor Moreau. C.A. Prieur-Duvernois, and Antoine Joseph Santerre. In addition, the collection includes a letter from the Danish physicist Hans Christian Oersted to Sir John Herschel, a letter by the French poet Romain Rolland, a document of the Philadelphia Artists' Fund Society of 1846 with signatures of its officers, and an autograph letter and a photograph of Henry Wadsworth Longfellow.