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Letters written by Dr. Watts, his family, friends, patients, and colleagues. There are also many documents including Dr. Watts' appointment as an army surgeon July 6, 1812 signed by President Madison. Included amongst the documents are announcements of faculty teas, meetings of the trustees, faculty letters, and a catalogue of the officers and students of Columbia College, 1867-1868.

Correspondence, manuscripts of poems, and manuscripts of lectures by Benjamin. The correspondence consists of original letters of Benjamin, typescript and photostatic copies of Benjamin letters in other libraries, and letters to Benjamin from some of his literary contemporaries including Paul Hamilton Hayne, Willis Gaylord Clark, John Lothrop Motley, and Fitz-Greene Halleck. Many of the letters relate to Park Benjamin's lecture tours. There are other family letters and many documents relating to the Benjamin family,and two letterbooks of John Lothrop Motley. Also, a large amount of genealogical material of the Benjamin family, and its related families from the 16th century to the present day. There are also financial records, monographs, clippings, and photographs.

Correspondence, documents and manuscripts from late seventeenth and eighteenth century France, especially from the French Revolution, collected by Sam Schaefler. Authors include J.B. Colbert Torcy and the Duchesse Du Lude. Many of the items from the French Revolution represent the work of the Committee of Public Safety and the Committee of General Security. French Revolutionary leaders represented in the collection include François-Antoine Boissy D'Anglas, Jean-Baptiste-Noel Bouchotte, Pierre Joseph Cambon, Lazare Carnot, Jean-Marie Collot D'Herbois, l'Abbʹe de Fauchet, Philippe-Antoine Merlin de Douai, Jean Victor Moreau. C.A. Prieur-Duvernois, and Antoine Joseph Santerre. In addition, the collection includes a letter from the Danish physicist Hans Christian Oersted to Sir John Herschel, a letter by the French poet Romain Rolland, a document of the Philadelphia Artists' Fund Society of 1846 with signatures of its officers, and an autograph letter and a photograph of Henry Wadsworth Longfellow.