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The collection contains correspondence, memoranda, drafts, committee meeting reports, speeches, calendars, etc. of Grayson L. Kirk, former Columbia University President. Also included are books from his library. There are also materials deemed by the Office of the President staff as "personal," meaning not directly related to Columbia University. These included the records of the Jacob R. Schiff Charitable Trust and the New York World's Fair 1964-1965.

The collection includes 21 posters relating to book arts, and a number of historical rare book dealer and auction catalogs and booklets related to rare book librarianship. It also includes several groups of printed materials, documents, art and memorabilia related to literature, performing arts, and the New York World's Fairs of 1939-40 and 1964-65.

This image collection consists of one black leather album containing 105 archive-quality 5x7 inch historic photos (of which 90 are manually darkroom-produced, black-and-white enlargements, mainly from negatives) depicting Columbia College student life and related current events during 1963-1965, plus photo captions totaling about 1,800 words. Also 4 CDs totaling 39 digitally reproduced color and B&W images.