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More than 120 architects from the United States and abroad contributed original drawings to this collection. Most are hand-drawn; some are printed through traditional etching or lithography techniques; a few others are computer-generated prints. Images are primarily related to the architects' projects, although some drawings are travel sketches of other structures. Drawings in this archive were exhibited at the Miriam & Ira D. Wallach Art Gallery and the Arthur Ross Gallery at Columbia University, Apr. 3-May 4, 1991. At least one drawing from each contributor was published in the accompanying exhibition catalog, CONTEMPORARY ARCHITECTURAL DRAWINGS (San Francisco: Pomegranate Artbooks, 1991).

This collection is photograph archive of the works of architectural photographer George Cserna. Images include interior and exterior shots of prominent New York buildings primarily during the 1960s. The collection has been arranged alphabetically by the client or architect of the building. Some of George Cserna's most notable work in this collection includes photographs of Ulrich Franzen's Agronomy Building, Emerson Hall, and Goddard Library at Cornell University; Haines, Lundberg, and Waehler's U.S. Trust Building and Schering-Plough Headquarters; Victor Lundy's I. Miller Store and IBM Headquarters; and I. M. Pei's John Hancock Tower, Mount Royal Bank and Ville Marie Complex, and MIT Chemistry Building. The collection also contains photographs of exhibitions and openings at the Museum of Modern Art in the 1960s and 1970s, such as The Responsive Eye and Toward a Rational Automobile. Finally, the collection has photographic portraits of notable persons including John dos Passos, W.H. Auden, and William Faulkner.

The materials that comprise the Historical Biographical Files have been collected and added to from a variety of sources over the years by current and previous staff. The files consist of materials related to people who have a connection to the University whether as student, alumni, administrator, faculty, staff, guest lecturer, or honorary degree recipient. Materials generally consist of newspaper and magazine clippings, press releases, programs, ephemera, printed matter, lists, reports, and pamphlets.

The bulk of this collection consists of more than 22,000 black and white photographic negatives and more than 10,600 black and white photographic prints documenting commercial, institutional, religious, and residential architecture throughout the United States, with particular emphasis on sites in the mid-Atlantic region. These images date from the mid-1930s to Molitor's retirement in the mid-1980s, with the great majority of images created between 1946 and 1980. Also included in the collection are images of landscapes, industrial design, portraits, and events of personal significance to Molitor. In some select cases, color prints, color negatives, color transparencies, and 35mm slides are also available in addition to or instead of the black and white negatives and prints. Researchers are also advised that documents in this collection indicate that when faced with a lack of storage space in 1973, Molitor contacted clients to return inactive negatives that they had comissioned before 1955. In at least some cases, those clients declined to accept their negatives and Molitor subsequently destroyed the images. Thus, this collection has lacunae in the negatives series.