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The large collection covers all aspects of Cordier's life. It contains letters, memoranda, reports, cables, printed materials and photographs, mostly pertaining to his tenure at the United Nations and Columbia University.

The correspondence, research, and teaching files of French-American cultural historian and Columbia University professor emeritus Jacques Barzun (1907-2012).

The V. K. Wellington Koo papers document the diplomatic legacy of Wellington Koo as a Chinese statesman and diplomat of the 20th Century. The papers primarily consist of materials collected during Koo's diplomatic career, relating to the Lytton Commission, 1932-1933; the League of Nations, 1931-1940; the United Nations, 1944-1946; his ambassadorships to France, 1932-1941; to Britain, 1941-1946; to the United States, 1946-1956; as the Senior Advisor to the Republic of China from 1956; and as the Judge on the International Court of Justice, 1957-1966. The materials include correspondence, diaries, memoranda, manuscripts, documents, notes, speeches, maps, photographs, printed material, and audio visual material. The bulk of the materials emphasizes China's domestic and foreign affairs, such as the Sino-Japanese conflict, World War II and the Cold War in the Far East region, as well as the League of Nations and the United Nations.

The Wallace K. Harrison architectural drawings and papers consists of architectural drawings, photographs, correspondence, notes, speeches, manuscripts, press releases, clippings, memoranda, printed material, job lists, curriculam vitae, contracts, articles, and other material related to Harrison's architectural projects. The collection also contains a significant amount of material regarding Harrison's position as director of the Office of Inter-American Affairs, director of planning of the United Nations Headquarters and biographical material. Approximately a third of the collection is made up of photographs. Photographers include Wendy Barrows, Shirley Burden, George Cserna, Y[uzo] Nagata, and Ezra Stoller, among many others. There is also a collection of 148 art books that belonged to Harrison referred to as his "doodle books." A list of these books with brief descriptions of where Harrison drew in them is contained in the finding aid. Projects documented include Lincoln Center, Metropolitan Opera House, Rockefeller Center, Albany Mall (Empire State Plaza), United Nations, X City, ALCOA building, Corning Glass building, First Presbyterian Church, La Guardia Airport, Socony-Mobil building, Battery Park City, Radio City Music Hall, New York World's Fair (1939 and 1964), Institute for Advanced Study, National Academy of Science, Pahlavi National Library Competition, Oberlin College's Hall Auditorium, Pershing Memorial, Rockefeller University, Hopkins Center, The Anchorage, Avila Hotel, and numerous other buildings and residences.