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Papers concerning both the administration of the Henry Street Settlement and Wald's involvement in numerous philanthropic and liberal causes. Her office files trace the foundation and growth of the Henry Street Settlement from 1895 until 1933. Her other activities include child welfare, civil liberties, immigration, public health, unemployment, and the peace movement during World War I. The correspondence files contain letters from public figures and writers including Jane Addams, Roger N. Baldwin, Van Wyck Brooks, Lavinia L. Dock, John Galsworthy, Samuel Gompers, William D. Howells, Charles Evans Hughes, Mabel Hyde Kittredge, Frances Perkins, Dorothy Thompson, Norman Thomas, Ida Tarbell, Margaret Sanger, and Jacob A. Riis.

The collection consiste of correspondence, memoranda, reports, bulletins, clippings, photographs, awards, and printed material. The files, arranged by genre and topic and reflect her philanthropic and legislative work in the areas of health, specifically cancer, heart disease, and mental health. Her civic and legislative work is covered in detail, as well as her private interests and activities.