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The collection contains correspondence with the authors, including contracts signed with authors as well as negotiations with the authors over various aspects of publishing their works; financial records documenting many aspects of the operation of Harper & Brothers, including royalties paid to authors, records of stock offerings and company reorganizations, and general ledgers which contain daily notes on all aspects of the operation of the business; book catalogues and trade lists; research materials collected by Eugene Exman for his history of Harper & Brothers; visual materials, from drawings and photographs of Harper's authors to colophon designs and an oil painting of the original Harper's building.

Correspondence, manuscripts of poems, and manuscripts of lectures by Benjamin. The correspondence consists of original letters of Benjamin, typescript and photostatic copies of Benjamin letters in other libraries, and letters to Benjamin from some of his literary contemporaries including Paul Hamilton Hayne, Willis Gaylord Clark, John Lothrop Motley, and Fitz-Greene Halleck. Many of the letters relate to Park Benjamin's lecture tours. There are other family letters and many documents relating to the Benjamin family,and two letterbooks of John Lothrop Motley. Also, a large amount of genealogical material of the Benjamin family, and its related families from the 16th century to the present day. There are also financial records, monographs, clippings, and photographs.