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Correspondence, memoranda, photographs, manuscripts, lists, legal and financial documents, and printed materials of Simon. The personal and business papers include correspondence with authors, inscribed photographs of authors, editorial files, files for his special art, photography, and music projects, correspondence files relating to Simon and Schuster, Inc., personal and family correspondence, documents, and photographs. Correspondents include Irving Berlin, Margaret Bourke-White, Henri Cartier-Bresson, Joseph E. Davies, Dwight D. Eisenhower, Philippe Halsman, Jerome Kern, Cole Porter, Kenneth Roberts, Arthur Schnitzler, Jerome Weidman, and Sloan Wilson.

Correspondence, subject files, corporate committee files, corporate reports, yearly appointment calendars, biographical materials, photographs, books from his personal library, memorabilia and works of art. Correspondence includes 3 bound slipcased volumes containing 471 letters, notes and congratulatory telegrams on the occasion of R.D. Lilley being named President of AT&T, April 1, 1972. Correspondents include David Rockefeller and Peter W. Rodino, Jr. Subject files contain Columbia University activities. Manuscript files include his student notebooks from the School of Engineering (1931) and the School of Mines (1934-1935). Corporate committee files include the New Jersey Commission on Civil Disorders, 1967-1968. Memorabilia consists of seven Columbia University related plaques, awards, citations, and varsity letters and fifteen Columbia related commemorative gifts and tokens, as well as thirty-five non-Columbia related diplomas, plaques, awards, citations and certificates and fifty-five non Columbia related trophies, commemorative gifts, and presentation pen & pencil sets. The works of art include two views of the Park Place building "Columbia College New-York" (NEW YORK MIRROR, 1828) and "Columbia College and College Green" (New York, 1830) facsimile reprint of the "Palm tree print"; a print of a drawing of "Columbia University circa 1903" from the Avery Library; two signed prints of Ernest D. Roth "Hamilton Hall" and the "School of Mines"; and a relief print of "John Jay" by Stanley Wyatt.

The records of W.R. Grace & Co. cover the rise of the Grace shipping business from 1864 until World War II. The early correspondence concerns all aspects of the shipping business in New York and South America, mining interests in Peru and Chile, the railroad in Costa Rica, the inter-ocean canal planned for Nicaragua, and political interests throughout Central and South America. There are letter books, correspondence, and scrapbooks of clippings for all aspects of W.R. Grace's career. There are minute books and other documents for more than 50 subsidiary companies owned by W.R. Grace & Co. or by family members. The papers of Joseph Peter Grace (1872-1950) continue the business, family, and philanthropic activities until 1942. There are also 20 reels of motion picture film about the Grace Co. South American interests in the 1950s.